The basic principle of fast-charging LIBs is to achieve fast Li + transport in both electrode and electrolyte as well as the electrode/electrolyte interfaces.
In future, the development of advanced characterization techniques such as Cyro-TEM, synchrotron X-ray analysis is expected to reveal more new light on the fast-charging technology. As the “blood” of LIBs, it’s doubtless that regulating the properties of electrolytes is an essential strategy to enhance the fast-charging performance.
To enable their application in fast-charging systems, modification approaches including the design of nanostructures to mitigate volume change , , integration with carbon materials to enhance Li + transport kinetics , and surface modifications , to prevent the interface side reactions are commonly used.
High intrinsic ionic conductivity and electrochemical stability are inherent requirements for solid-state electrolytes to be applied in fast-charging LIBs.
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